The g factors of 11/2− isomers in semimagic 109Sn and 111Sn (isomeric lifetimes τ=2.9(3) ns and τ=14.4(7) ns, respectively) were measured by an extension of the Time Differential Perturbed Angular Distribution technique, which uses LaBr3 detectors and the hyperfine fields of a gadolinium host to achieve precise measurements in a new regime of short-lived isomers. The results, g(11/2−;109Sn)=−0.186(8) and g(11/2−;111Sn)=−0.214(4), are significantly lower in magnitude than those of the 11/2− isomers in the heavier isotopes and depart from the value expected for a near pure neutron h11/2 configuration. Broken-symmetry density functional theory calculations applied to the sequence of 11/2− states reproduce the magnitude and location of this deviation. The g(11/2−) values are affected by shape core polarization; the odd 0h11/2 neutron couples to Jπ=2+,4+,6+... configurations in the weakly-deformed effective core, causing a decrease in the g-factor magnitudes.

The A≈100 mass region is of special interest due to a rapid shape transition, observed by going from neutron number 58 to 60, especially pronounced in the Zr isotopes, where 98Zr is weakly and 100Zr is strongly deformed. To further examine this intricate phenomenon, in this work lifetimes of low-lying excited states in the nuclei 99Zr and 99Nb were determined using fast-timing techniques and an experimental setup consisting of four LaBr3(Ce) detectors. Neutron rich A=99 fragments were produced in neutron induced fission and separated by the spectrometer LOHENGRIN at the Institut Laue-Langevin in Grenoble, France. Experimental values are compared to two different calculations in the framework of the interacting boson-fermion model and discussed in the context of shape coexistence.